Comment They'd serve different purposes. (Score 2) 8
A balloon is not static, it moves with the atmospheric system it is in. Ergo, it tells you how that system evolves. A drone cannot do this.
A drone can stay put, relative to the ground, telling you how a location's atmosphere evolves. A balloon cannot do this.
These are solving completely different types of problem.
You could, of course, construct a hybrid, as balloons are traditionally single-shot. If a balloon carries the measurement gear and a drone capable of carrying that same gear PLUS a deflated balloon, then you can have something that operates as a balloon until it reaches some pre-set location, whereupon the balloon's gas is released and the drone flies the ensemble to a collection point.