Nickel-64, at a natural abundance of about 1%, would be a better candidate, as neutron capture would result in Nickel-65 which decays to stable Copper-65 with a very short half-life of 2 hours. This is a "clean" beta-emitter with an energy of about 2.1MeV.
The overall reaction seems to be p + Ni-64 -> Cu-65 + ve + anti-ve + 2.1MeV. This is at least physically plausible as a reaction. The electron (removed from both sides above) acts as a sort of catalyst, a way to get the proton through the coloumb barrier by transforming it into a neutron.
Getting the neutrons to collide with Ni-64 nuclei rather than escaping implies a lot of Ni-64, and any escaping neutrons would irradiate everything else nearby, or impurities in the nickel such as the aforementioned Ni-62, or worse Ni-58 which would produce Ni-59, a positron emitter with a half-life of 76000 years.
But to me, the real red flag on this is getting the hydrogen atoms to collapse into neutrons, a process which I've never heard of before. Even if it's possible, can you get a net gain? Does it take more than 2.1MeV? Slashdot - educate me!