If you look at the absorption and efficiency plots in the linked nature abstract, the improvement is pretty broad spectrum as it is. Based on the Fourier analysis plots, it does seem like a slightly wider pit spacing would better concentrate the energy in their desired sweet spot, but CDs and DVDs would be too wide. HD-DVD actually looks like it might have the most ideal pit spacings.
Now that they have a proof of concept, it is an obvious thing for researchers to try different pit sizes and patterns in order to optimize the efficiency
Actually, that already happened. As the abstract of the paper notes, previous research has already identified how to theoretically optimize patterns, but arbitrary patterns require expensive photo lithography equipment to create. This research shows that an existing inexpensive mass production technique generates results that are almost as good as the optimized patterns, but not quite as good because the spacing of the pits is a bit too periodic (especially across tracks rather than along them).
...it wasn't the first computer.
I tell them to turn to the study of mathematics, for it is only there that they might escape the lusts of the flesh. -- Thomas Mann, "The Magic Mountain"